厦门大学化学化工学院催化科学与工程研究所王勇

sujue

王勇
教授、博士生导师
电子邮箱：wang42@xmu.edu.cn;  yongwangwausa@hotmail.com
课题组网页：http://121.192.177.81:90/ywang/index.html
个人简历：
硕士：（美国华盛顿州立大学，1992年）
博士：（美国华盛顿州立大学，1993年）
2009年入选中组部##计划
研究兴趣：
先进催化材料和新型反应器
碳资源中间体包括合成气的转化
近期主要代表论著：
2016
1.J.Jones, H.Xiong, A.T. DeLaRiva, E.J. Peterson, H.Pham, S.R. Challa, G.Qi, S.Oh, M.H. Wiebenga, X.Hernández, Y.Wang, A.K. Datye, “Thermallystable single-atom platinum-on-ceria catalysts via atomtrapping”, Science, 2016, 353(6295), 150-154. doi: 10.1126/science.aaf8800
2.M.Pruski, A.D. Sadow, I. I. Slowing , C. L. Marshall, P.Stair, J.Rodriguez, A. Harris , G. A. Somorjai , J.Biener , C. Matranga, C.Wang , J. A. Schaidle, G.T. Beckham, D.A. Ruddy, T.Deutsch, S.M. Alia , C.Narula, S.Overbury, T.Toops , R. M.Bullock, C.H. F. Peden, Y.Wang , M.D. Allendorf , J.N?rskov, T.Bligaard, Preface of Virtual Special Issue on Catalysis at the U.S. Department of Energy’s National Laboratories, ACS Catalysis, 2016, 3227–3235, doi: 10.1021/acscatal.6b00823
3.W.Wang, K.Wu, P.Liu, L.Li, Y.Yang, Y.Wang, “Hydrodeoxygenation of p-Cresol over Pt/Al2O3 Catalyst Promoted by ZrO2, CeO2, and CeO2-ZrO2”, Ind.Eng.Chem.Res., 2016, doi: 10.1021/acs.iecr.6b00515
4.Y.Hong, A.Hensley, J.S.McEwen, and Y.Wang, “Perspective on pyrolysis of biomass: essential roles of Fe based bimetallic catalysts”, Catal.Lett. 2016, doi: 10.1007/s10562-016-1770-1 (invited perspective).
5.Lei Du, Yuyan Shao, Junming Sun, Geping Yin, Jun Liu, Yong Wang, “Advanced catalyst supports for PEM fuel cell cathodes” Nano Energy, 2016, doi:10.1016/j.nanoen.2016.03.016.
6.Changjun Liu, Junming Sun, Heather M. Brown, Oscar G. Marin-Flores, Tim Bays, Ayman M. Karim, and Yong Wang “Aqueous Phase Hydrodeoxygenation of Polyols over Pd/WO3-ZrO2: Role of Pd-WO3 Interaction and Hydrodeoxygenation Pathway” Catalysis Today 2016, 269, 103-109. doi: 10.1016/j.cattod.2015.10.034
7.Stephen Davidson, Junming Sun, Yong Wang “The effect of ZnO addition on H2O activation over Co/ZrO2 catalyst”,Catalysis Today 2016, 269, 140-147. doi: 10.1016/j.cattod.2015.10.016
8.Rebecca A.L. Baylon, Junming Sun, Kevin J. Martin, Padmesh Venkitasubramanian and Yong Wang “Beyond ketonization: selective conversion of carboxylic acids to olefins over balanced Lewis acid–base pairs”, Chemical Communications, 2016, 52, 4975-4978. doi: 10.1039/C5CC10528E
9.Junming Sun, Rebecca A.L. Baylon, Changjun Liu, Donghai Mei, Kevin J. Martin, Padmesh Venkitasubramanian and Yong Wang “Key roles of Lewis Acid-Base Pairs on ZnxZryOz in Direct Ethanol/Acetone to Isobutene Conversion” Journal of the American Chemical Society, 2016, 2, 507-517. doi: 10.1021/jacs.5b07401
10.Mahfuzur M. Rahman, S. Davidson, Junming Sun, Yong Wang “Effect of water on ethanol conversion on ZnO”, Topics in Catalysis, 2016, 59, 37-45. doi: 10.1007/s11244-015-0503-9
11.Ning Yu, He Zhang, Stephen Davidson, Junming Sun, Yong Wang* “The effect of ZnO facets on ethanol steam reforming on Co/ZnO”, Catalysis Communications, 2016, 73, 93. doi: 10.1016/j.catcom.2015.10.018
12.Rebecca A.L. Baylon, Junming Sun, Yong Wang “Conversion of Ethanol to 1, 3-Butadiene over Na doped ZnxZryOz Mixed Metal Oxides” Catalysis Today, 2016, 259, 446-452. doi: 10.1016/j.cattod.2015.04.010
13.Jian Zhi Hu, Suochang Xu, Ja Hun Kwak, Mary Y Hu, Chuan Wan, Zhenchao Zhao, Janos Szanyi, Xinhe Bao, Xiuwen Han, Yong Wang, Charles HF Peden “High field 27 Al MAS NMR and TPD studies of active sites in ethanol dehydration using thermally treated transitional aluminas as catalysts” Journal of Catalysis, 2016, 336, 85-93. doi: 10.1016/j.jcat.2016.01.006
14.C.Miao, O.Marin-Flores, S.Davidson, T.Li, D.Tao, D.Gao, Y.Wang, M.Garcia-Perez, S.Chen, “Hydrothermal catalytic deoxygenation of palmitic acid over nickel catalyst”, Fuel, 2016, 166(15): 302-308, doi: 10.1016/j.fuel.2015.10.120.
2015
1.Y.Shao, Y.Cheng, W.Duan, W.Wang, Y.Lin, Y.Wang*, J.Liu*, “Nanostructured electrocatalysts for PEM fuel cells and redox flow batteries: a selected review”, ACS Catalysis, 2015, doi:10.1021/acscatal.5b01737
2.A.Hensley, Y.Wang, J.S.McEwen, “Adsorption of Guaiacol on Fe (110) and Pd (111) from First Principles”, Surface Science, 2015, doi:10.1016/j.susc.2015.10.030.
3.Z.Wei, A.Karim, Y.Wang, “Elucidation of the roles of Re in aqueous-phase reforming of glycerol over Pt-Re/C catalysts”,ACS Catalysis, 2015, doi: 10.1021/acscatal.5b01770.
4.H.Wang, Y.Wang, “Characterization of deactivated bio-oil hydrotreating catalysts”, Topics in Catalysis. 2015, doi: 10.1007/s11244-015-0506-6.
5.K.K.Ramasamy, M.Gray, H.Job, D.Santosa, S.X.Li, A.Devaraj, A.Karkamkar, Y.Wang, “Role of calcination temperature on the hydrotalcite derived MgO-Al2O3 in converting ethanol to butanol”, Topics in Catalysis. 2015. doi: 10.1007/s11244-015-0504-8.
6.Z.Fang, Y.Wang, D.A.Dixon, “Computational Study of Ethanol Conversion on Al8O12 as a Model for γ-Al2O3”, JPCC. 2015, 119:23413–23421, doi: 10.1021/acs.jpcc.5b05887.
7.Z.Chase, A.Vjunov, J.L.Fulton, D.M.Camaioni, M.Balasubramanian, Y.Wang, J.A.Lercher, “State of supported Ni nanoparticles during catalysis in aqueous media”, Chemistry-A European Journal. 2015, doi: 10.1002/chem.201502723.
8.J.Sun, A.Karim, X.Li, Y.Shin, Y.Wang, “Hierarchicaqlly structured catalysts for cascade and selective steam reforming/Hydrodeoxygenation reactions”, Chem.Comm, 2015, doi: 10.1039/C5CC07244A.
9.J.Sun, S.Wan, F.Wang, J.Lin, Y.Wang, “Selective synthesis of methanol and higher alcohols over Cs/Cu/ZnO/Al2O3catalysts”, Ind.Eng.Chem.Res., 2015, doi: 10.1021/acs.iecr.5b01927.
10.H.Zhang, J.Sun, C.Liu, Y.Wang, “Distinct water activation on polar/non-polar facets of ZnO nanoparticles”, J.Catal, 2015, doi: 10.1016/j.jcat.2015.08.016.
11.A.Hensley, S.Schneider, Y.Wang, J.S.McEwen, “Adsorption of aromatics on the (111) surface of PtM and PtM3 (M=Ni, Fe) alloys”, RSC Advances, 2015, doi: 10.1039/c5ra13578h.
12.W.Li, F.Gao, Y.Li, J.Liu, C.H.F.Peden, Y.Wang,”Nanocrystalline anatase titania supported vanadia catalysts: facet-dependent structure of vanadia”, J.Phy.Chem C, 2015, doi: 10.1021/acs.jpcc.5b01486.
13.J.Sun, H.Zhang, Y.Ning, S.Davideson, Y.Wang, “Effect of cobalt particle size on acetone steam reforming”, ChemCatChem,2015, doi: 10.1002/cctc.201500336
14.R.A.L.Baylon, J.Sun, Y.Wang, “Conversion of ethanol to 1,3-butadiene over Na doped ZnxZryOz mixed metal oxides”,Catalysis Today, 2015, doi: 10.1016/j.cattod.2015.04.010.
15.J.Hu, S.Xu, W.Li, M.Hu, X.Deng, D.Dixon, M.Vasiliu, R.Craciun, Y.Wang, X.Bao, C.H.F.Peden, “Investigation of the structure and active sites of TiO2 nano-ro supported VOx catalysts by high field and fast spinning 51V MSA NMR”, ACS Catalysis, 2015, doi: 10.1021/acscatal.5b00286.
16.K.K.Ramasamy, M.Gray, H.Job, Y.Wang, “Direct syngas hydrogenation over a Co-Ni bimetallic catalyst: process parameter optimization”, Chem.Eng.Sci., 2015, doi: 10.1016/j.ces.2015.03.064
17.Y.Li, Z.Wei, F.Gao, L.Korarik, R.Long, C.H.F.Peden, Y.Wang, “Effect of oxygen defects on the catalytic performance of VOx/CeO2 catalysts for oxidative dehydrogenation of methanol”, ACS Catalysis, 2015, doi: 10.1021/cs502084g.
18.J.D.Holladay, Y.Wang, “3-D model of a radial flow sub-watt methanol fuel processor”, Chem.Eng.Sci., 2015, doi: 10.1016/j.ces.2015.02.012.
19.J.D.Holladay, Y.Wang, “A review of recent advances in numerical simulations of microscale fuel processor for hydrogen production”, Journal of Power Sources, 2015, doi: 10.1016/j.jpowsour.2015.01.079
20.Z. Wei, A. Karim, Y. Li, D.L. King, Y. Wang. “Elucidation of the roles of Re in steam reforming of glycerol over Pt-Re/C catalysts”, J.Catal., 2015, 322, 49–59. doi: 10.1016/j.jcat.2014.11.006.
21.H. Xiong, A. Riva, Y. Wang, A. Datye. “Low-temperature aqueous-phase reforming of ethanol for CO-free H2 production on bimetallic PdZn catalyst”, Catalysis Science & Technology, 2015, 5, 254–263. doi: 10.1039/c4cy00914b.
22.J. Sun, A.M. Karim, D. Mei, M. Engelhard, X. Bao, Y. Wang, “New insights into reaction mechanisms of ethanol steam reforming on Co-ZrO2”, Applied Catalysis B: Environmental, 2015, 162, 141–148. doi: 10.1016/j.apcatb.2014.06.043
2014
1.Y.Shao, N.Rjput, J.Hu, M.Hu, T.Liu, Z.Wei, M.Gu, X.Deng, S.Xu, K.S.Han, J.Wang, Z.Nie, G.Li, K.R.Zavadil, J.Xiao, C.Wang, W.A.Henderson, J.G.Zhang, Y.Wang, K.T.Mueller, K.Persson, J.Liu, “Nanocomposite polymer electrolyte for rechargeable magnesium batteries”, Nano Energy, 2014, doi:10.1016/j.nanoen.2014.12.028.
2.O.G.Marin-Flores, A.Karim, Y.Wang, “Role of tungsten in the aqueous phase hydrodeoxygenation of ethylene glycol on tungstated zirconia supported palladium”, Catalysis Today, 2014, 237, 118-124, doi: 10.1016/j.cattod.2014.03.068.
3.A.J.R. Hensley, Y. Wang, J.S. McEwen. “Phenol deoxygenation mechanisms on Fe(11) and Pd(111)”, ACS Catalysis, 2014. (accepted) doi: 10.1021/cs501403w
4.V.M. Dagle, R.A. Dagle., J. Li, C. Deshmane, D.E. Taylor, X. Bao, Y. Wang. “Direct conversion of syngas-tohydrocarbons over higher alcohols synthesis catalysts mixed with HZSM-5”, Ind.Eng.Chem.Res., 2014, 53 (36), pp 13928-13934. doi: 10.1021/ie502425d
5.A.J.R. Hensley, Y. Wang, J.S. McEwen. “Adsorption of Phenol on Fe (110) and Pd (111) from First Principles”, Surface Science, 2014, 630, 244–253. doi: 10.1016/j.susc.2014.08.003.
6.W. Li, L. Kovarik, D. Mei, M.H. Engelhard, F. Gao, J. Liu, Y. Wang, C.H.F. Peden. “A general mechanism for stabilizing the small sizes of precious metal nanoparticles on oxide supports”, Chemistry of Materials, 2014, 26 (19), 5475–5481. doi: 10.1021/cm5013203.
7.A.J.R. Hensley, Y. Hong, R. Zhang, H. Zhang, J. Sun, Y. Wang. J.S.McEwen, “Enhanced Fe2O3 reducibility via surface modivication with Pd: characterizing the synergy within Pd/Fe catalysts for hydrodeoxygenation reactions”, ACS Catalysis, 2014, 4 (10), 3381–3392. doi: 10.1021/cs500565e.
8.A.K. Dalai, Y. Wang. Preface, Catalysis Today, 2014, 237, 1–2.
9.Yang Y., J.S. Dennis, M. Saeys, Y. Wang. Preface, Catalysis Today, 2014, 233, 1.
10.Y. Li, Z. Wei, Y. Wang. “Ni/MgO Catalyst Prepared via Dielectric-Barrier Discharge Plasma with Improved Catalytic Performance for Carbon Dioxide Reforming of Methane”, Frontiers of Chemical Sciences and Engineering, 2014, 8 (2), 133–140. doi: 10.1007/s11705-014-1422-1.
11.J. Sun, Y. Wang. “Review of ethanol conversion to chemicals and fuels”, ACS Catalysis, 2014, 4 (4), 1079–1090. doi: 10.1021/cs4011343. (featured on cover of the 2014 April issue).
12.J. Kwak, R. Dagel, G. Tustin, J. Zoeller, L. Allard, Y. Wang. “Molecular active sites in heterogeneous Ir-La/C catalyzed carbonylation of methanol to acetates”, J.Phy.Chem.Lett., 2014, 5 (3), 566–572. doi: 10.1021/jz402728e
13.H. Zhang, J. Sun, V.L. Dagle, B. Halevi, A.K. Datye, Y. Wang, “Influence of ZnO Facets on Pd/ZnO Catalysts for Methanol Steam Reforming”, ACS Catalysis 2014, 4 (7), 2379–2386. doi: 10.1021/cs500590t
14.Y-C Hong, H. Zhang, J. Sun, A.M. Karim, A.J.R. Hensley, M. Gu, M.H. Engelhard, J-S McEwen, Y. Wang, “Synergistic Catalysis between Pd and Fe in Gas Phase Hydrodeoxygenation of m-Cresol”, ACS Catalysis, 2014, 4 (10), 3335–3345. doi: 10.1021/cs500578g
15.S.D. Davidson, J. Sun, Y-C Hong, A.M. Karim, A.K. Datye, Y. Wang, “The effect of ZnO addition on Co/C catalyst for vapor and aqueous phase reforming of ethanol”, Catalysis Today, 2014, 233, 38–45. doi: 10.1016/j.cattod.2013.12.044
16.K.Ramasamy, Y.Wang, “Ethanol conversion on HZSM-5: effect of reaction conditions and Si/Al ratio on the product distributions”, Catalysis Today, 2014, 237, 89–99. doi: 10.1016/j.cattod.2014.02.044.
17.O.G.Marin-Flores, A.Karim, Y.Wang, “Role of tungsten on the catalytic performance of tungstated zirconia supported palladium for the aqueous phase hydrodeoxygenation of ethylene glycol”, Catalysis Today, 2014, 237, 118–124. doi: 10.1016/j.cattod.2014.03.068.
18.S.Wan and Y.Wang, “A review on ex situ catalytic fast pyrolysis of biomass”, Frontiers of Chemical Science and Engineering, 2014. 8 (3): 280–294. doi: 10.1007/s11705-014-1436-8
19.C.Liu, H.Wang, A.Karim, J.Sun, Y.Wang, “Advances in catalytic pyrolysis of lignocellulosic biomass”, Chem.Soc.Rev., 2014,43, 7594–7623. doi: 10.1039/c3cs60414d (invited review)
20.Y.Li, Z.Wei, F.Gao, L.Kovarik, C.H.F.Peden, Y.Wang, “Effects of CeO2 Support Facets on VOx/CeO2 Catalysts in Oxidative Dehydrogenation of Methanol”, Journal of Catalysis, 2014, 315, 15–24. doi: 10.1016/j.jcat.2014.04.013
21.S.Davison, J.Sun, H.Zhang, Y.Wang, “Supported metal catalysts for alcohol/sugar alcohol steam reforming”, Dalton Transactions, 2014, 43, 11782–11802. doi: 10.1039/c4dt00521j (invited perspective, cover of the issue 31 of 2014).
22.K.Ramasamy, H.Zhang, J.Sun, Y.Wang, “Performance of hierarchical HZSM-5 for the conversion of ethanol to hydrocarbon”, Catalysis Today, 2014, 238, 103–110. doi: 10.1016/j.cattod.2014.01.037.
2013
1.W. Li, L. Kovarik, D. Mei, J. Liu, Y. Wang, C.H.F. Peden, "Anti-sintering Pt nanoparticles stabilized by MgAl2O4 spinel {111} facets", Nature Communications, 2013. doi: 10.1038/ncomms3481
2.Z. Chase, J. Fulton, D. Camaioni, D. Mei, M. Balasubramanian, V. Pham, C. Zhao, R. Weber, Y. Wang, J. Lercher, "State of Supported Pd during Catalysis in Water", J.Phy.Chem.C, 2013. doi: 10.1021/jp404772p
3.K.K. Ramasamy, M.A. Gerber, M. Flake, H. Zhang, Y. Wang, "Conversion of biomass-derived small oxygenates over HZSM-5 and its deactivation mechanism", Green Chemistry, 2013. doi: 10.1039/c3gc41369a
4.V.M. Lebarbier, R.A. Dagle, L. Kovarick, K.O. Albrecht, C.E. Taylor, X. Bao, Y. Wang, "Sorption-enhanced synthetic natural gas from syngas: a novel process combining CO methanation, water-gas-shift, and CO2 capture", Appl. Catal. B, 2013. doi: 10.1016/j.apcatb.2013.06.03
5.C.Liu, J. Sun, C. Smith, Y.Wang, "A Study of ZnxZryOz Mixed Oxides for Direct Conversion of Ethanol to Isobutene",Applied Catalysis A, 2013, 467:91-97. doi: 10.1016/j.apcata.2013.07.011
6.J. Sun, A. Karim, H. Zhang, L. Kovarik, X. Shari Li, A.J. Hensley, J.-S. McEwen, Y. Wang, "Carbon Supported Bimetallic Pd-Fe Catalysts for Vapor-phase Hydrodeoxygenation of Guaiacol" Journal of Catalysis 2013, 306, 47–57. doi: 10.1016/j.jcat.2013.05.020

chunxue

六方氮化硼(h-BN)是一种新型的高选择性催化丙烷氧化脱氢(ODHP)制烯烃的催化剂，除了生成丙烷，生成乙烯C2产物的选择性也高于C1产物。近日，厦门大学王勇和林敬东团队报道了ODHP在h-BN上与V基催化剂不一样的反应路径。实验发现，在h-BN催化剂上，丙烷C-C键断裂生成的甲基会发生氧化偶联生成C2产物，使得C2产物选择性高于C1产物。该工作不仅明确了N基催化剂催化ODHP的反应机理，而且为催化氧化其它烷烃反应提供了思路。

Jinshu Tian, Jingdong Lin*, Yong Wang*, et al. Propane oxidative dehydrogenation over highly selective hexagonalboron nitride catalysts: The role of oxidative coupling of methyl. ScienceAdvances, 2019.

DOI: 10.1126/sciadv.aav8063

http://advances.sciencemag.org/content/5/3/eaav8063?rss=1